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| Brad Pitt | Jesse James |
| Casey Affleck | Robert Ford |
| Sam Shepard | Frank James |
| Mary-Louise Parker | Zee James |
| Paul Schneider | Dick Liddil |
| Jeremy Renner | Wood Hite |
| Garret Dillahunt | Ed Miller |
| Zooey Deschanel | Dorothy Evans |
| Michael Parks | Henry Craig |
| Ted Levine | Sheriff Timberlake |
| Sam Rockwell | Charley Ford |
| Alison Elliott | Martha Bolton |
| James Carville | Gov. Crittenden |
| Tom Aldredge | Maj. George Hite |
| Kailin See | Sarah Hite |
Infamous and unpredictable, Jesse James plans his next big heist while he launches pre-emptive strikes against those looking to collect the reward the law has placed on his head, but the most deadly threat may come from those closest to him.
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