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| James Coburn | Sheriff Patrick J. Garrett |
| Kris Kristofferson | Billy the Kid |
| Bob Dylan | Alias |
| Jason Robards | Gov. Lew Wallace |
| Richard Jaeckel | Sheriff Kip McKinney |
| Katy Jurado | Mrs. Baker |
| Slim Pickens | Sheriff Colin Baker |
| Chill Wills | Lemuel |
| John Beck | John W. Poe |
| Rita Coolidge | Maria |
| R.G. Armstrong | Deputy Sheriff Bob Ollinger |
| Luke Askew | Eno |
| Richard Bright | Holly |
| Matt Clark | Deputy Sheriff J.W. Bell |
| Jack Dodson | Lewellen Howland |
| Jack Elam | Alamosa Bill/Kermit |
| Emilio Fernández | Paco |
| Paul Fix | Pete Maxwell |
| L.Q. Jones | Black Harris |
| Jorge Russek | Silva |
| Charles Martin Smith | Charlie Bowdre |
| Harry Dean Stanton | Luke |
| Claudia Bryar | Mrs. Horrell |
Garrett becomes a sheriff and hunts his old friend and associate, Billy
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