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| Steve McQueen | Henri ``Papillon'' Charriere |
| Dustin Hoffman | Louis Dega |
| Victor Jory | Indian chief |
| Don Gordon | Julot |
| Anthony Zerbe | Toussaint Leper Colony chief |
| Robert Deman | Maturette |
| Woodrow Parfrey | Clusiot |
| Bill Mumy | Lariot |
| George Coulouris | Dr. Chatal |
| Ratna Assan | Zoraima |
| William Smithers | Warden Barrot |
| Gregory Sierra | Antonio |
| Barbara Morrison | Mother Superior |
| Ellen Moss | Nun (uncredited) |
| Don Hanmer | Butterfly trader |
| Dalton Trumbo | Commandant (uncredited) |
Safecracker Henri ``The Butterfly'' Charriere tries to escape from Devil's Island with counterfeiter Louis Dega .
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