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| Hugh Grant | The Prime Minister |
| Laura Linney | Sarah |
| Colin Firth | Jamie Bennett |
| Alan Rickman | Harry |
| Bill Nighy | Billy Mack |
| Emma Thompson | Karen |
| Liam Neeson | Daniel |
| Martine McCutcheon | Natalie |
| Keira Knightley | Juliet |
| Rowan Atkinson | Rufus |
| Andrew Lincoln | Mark |
| Billy Bob Thornton | President of the United States |
| Joanna Page | Just Judy |
| Kris Marshall | Colin Frissell |
| Lúcia Moniz | Aurelia |
| Martin Freeman | John |
| Thomas Sangster | Sam |
| Heike Makatsch | Mia |
| Chiwetel Ejiofor | Peter |
| Rodrigo Santoro | Karl |
| Claudia Schiffer | Carol |
| Gregor Fisher | Joe |
| Olivia Olson | Joanna Anderson |
| Abdul Salis | Tony |
| Shannon Elizabeth | Harriet |
| Denise Richards | Carla |
| Sienna Guillory | Jamie's Girlfriend |
A prime minister, an office worker, a pop star, a jilted writer, married couples and various others deal with relationships in London.
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