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| Steve Carell | Maxwell Smart |
| Anne Hathaway | Agent 99 |
| Dwayne Johnson | Agent 23 |
| Alan Arkin | Chief |
| Terence Stamp | Siegfried |
| Terry Crews | Agent 91 |
| David Koechner | Agent Larabee |
| James Caan | The President |
| Bill Murray | Agent 13 |
| Patrick Warburton | Hymie |
| Masi Oka | Bruce |
| Nate Torrence | Lloyd |
| Ken Davitian | Shtarker |
| David S. Lee | Krstic |
| Dalip Singh | Dalip |
When members of the nefarious crime syndicate KAOS attack the U.S. spy agency Control, the Chief has to promote his eager analyst Maxwell Smart to field agent. Smart, partnered with veteran Agent 99, blends inexperience, enthusiasm and ineptitude as he works to thwart a world-domination plot hatched by the wily KAOS chief, Siegfried .
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